Shack-Hartmann Wavefront Sensing of Ultrashort Optical Vortices.

Light beams carrying Orbital Angular Momentum (OAM), also known as optical vortices (OV), have led to fascinating new developments in fields ranging from quantum communication to novel light-matter interaction aspects. Even though several techniques have emerged to synthesize these structured-beams, their detection, in particular, single-shot amplitude, wavefront, and modal content characterization, remains a challenging task. Here, we report the single-shot amplitude, wavefront, and modal content characterization of ultrashort OV using a Shack-Hartmann wavefront sensor. These vortex beams are obtained using spiral phase plates (SPPs) that are frequently used for high-intensity applications. The reconstructed wavefronts display a helical structure compatible with the topological charge induced by the SPPs. We affirm the accuracy of the optical field reconstruction by the wavefront sensor through an excellent agreement between the numerically backpropagated and experimentally obtained intensity distribution at the waist. Consequently, through Laguerre-Gauss (LG) decomposition of the reconstructed fields, we reveal the radial and azimuthal mode composition of vortex beams under different conditions. The potential of our method is further illustrated by characterizing asymmetric Gaussian vortices carrying fractional average OAM, and a realtime topological charge measurement at a 10Hz repetition rate. These results can promote Shack-Hartmann wavefront sensing as a single-shot OV characterization tool.

Towards subpicosecond pulses from solid target plasma based seeded soft X-ray laser.

We investigate the coherence of plasma-based soft X-ray laser (XRL) for different conditions that can alter the electron density in the gain region. We first measure the source temporal coherence in amplified spontaneous emission (ASE) mode. We develop a data analysis procedure to extract both its spectral width and pulse duration. These findings are in agreement with the spectral line shape simulations and seeded operation experimental results. Utilizing the deduced spectral width and pulse duration in a one-dimensional Bloch-Maxwell code, we reproduce the experimental temporal coherence properties of the seeded-XRL. Finally, we demonstrate efficient lasing in ASE and seeded mode at an electron density two times higher than the routine conditions. In this regime, using Bloch-Maxwell modeling, we predict the pulse duration of the seeded XRL to be ∼500fs.

One long and two short pumping pulses control for plasma x-ray amplifier optimization.

Development of efficient soft x-ray laser plasma amplifiers adapted to seeded operation, requires a better control over amplifier transverse spatial extent, brilliance control and gain lifetime. Here it is shown that pumping the plasma amplifier with one long and two short pump pulses (1L2S) provides advantages in terms of control for the specified parameters in the case of Ni-like Ag x-ray laser. Also, significant tunability of the gain lifetime in the 1L2S pumping scheme for Ne-like Ti x-ray laser is observed. Direct harmonics seeding and chirped harmonics seeding amplification approaches may benefit from the control of the gain lifetime, in terms of better use of the pump energy and as a way to reduce the amplified spontaneous emission in x-ray lasers.

Q-switched laser-assisted grazing incidence pumping (QAGRIP) for efficient soft x-ray laser generation.

We have investigated a new scheme for laser plasma transient collisional soft x-ray lasers based on the use of an additional laser to produce the preplasma. Soft x-ray emission measurements made for different solid targets are presented and discussed. A significant enhancement of the SXRL emission as compared to double-pulse single-beam grazing incidence (DGRIP) using the same pump laser is reported for 13.9- and 32.6-nm SXRL wavelengths.

Thin film beam splitter multiple short pulse generation for enhanced Ni-like Ag x-ray laser emission.

An alternative, novel multiple pulse generation scheme was implemented directly after the optical compressor output of an x-ray pump laser. The new method uses a polarization sensitive thin film beam splitter and a half-wavelength wave plate for tuning the energy ratio in the multiple short pulses. Based on this method, an extensive study was made of the running parameters for a grazing incidence pumped silver x-ray laser (XRL) pumped with a long pulse of 145 mJ in 6 ns at 532 nm and up to 1.45 J in few picoseconds at 810 nm. Fivefold enhancement in the emission of the silver XRL was demonstrated using the new pump method.

Enhanced high harmonic generation driven by high-intensity laser in argon gas-filled hollow core waveguide.

We show that a significant enhancement of the photon flux produced by high harmonic generation can be obtained through guided configuration at high laser intensity largely above the saturation intensity. We identify two regimes. At low pressure, we observe an intense second plateau in the high harmonic spectrum in argon. At relatively high pressure, complex interplay between strongly time-dependent ionization processes and propagation effects leads to important spectral broadening without loss of spectral brightness. We show that the relevant parameter for this physical process is the product of laser peak power by gas pressure. We compare source performances with high harmonic generation using a gas jet in loose focusing geometry and conclude that the source developed is a good candidate for injection devices such as seeded soft x-ray lasers or free electron lasers in the soft x-ray range.

Optimization of a tabletop high-repetition-rate soft x-ray laser pumped in double-pulse single-beam grazing incidence.

This Letter reports on the optimization of a tabletop nickel-like molybdenum transient collisionally excited soft x-ray laser (SXRL) at 18.9 nm performed by a double-pulse single-beam grazing incidence pumping (DGRIP). This scheme allows for the first time, to our knowledge, the full control of the pump laser parameters including the pre-pulse duration optimally generating the SXRL amplifier under a grazing incidence. The single-beam geometry of the collinear double-pulse propagation guarantees the ideal overlap of the pre-pulse and main pulse from shot to shot resulting in a more efficient and highly stable SXRL output. SXRL energies up to 2.2 microJ are obtained with a total pump energy less than 1 J for several hours at a 10 Hz repetition rate without realignment under once optimized double pumping pulse parameters including energy ratio, time delay, pre-pulse and main pulse durations, and line focus width.

Submicrometer digital in-line holographic microscopy at 32 nm with high-order harmonics.

Soft-x-ray digital in-line microscopic holography is achieved using a fully coherent high-order harmonic source emitting at 32 nm. Combination of commercial-grade soft-x-ray optics and a back-illuminated CCD detector allows a compact and versatile holographic setup. Different experimental geometries have been tested by imaging calibrated 50 nm tips and 1 microm wires. Spatial resolution of 800 nm is measured with magnifications ranging from 30 to 110 and a numerical aperture around 0.01. Finally, the potentiality of three-dimensional numerical reconstruction from a single hologram acquisition is shown experimentally.

Design and characterization of extreme-ultraviolet broadband mirrors for attosecond science.

A novel multilayer mirror was designed and fabricated based on a recently developed three-material technology aimed both at reaching reflectivities of about 20% and at controlling dispersion over a bandwidth covering photon energies between 35 and 50 eV. The spectral phase upon reflection was retrieved by measuring interferences in a two-color ionization process using high-order harmonics produced from a titanium: sapphire laser. We demonstrate the feasibility of designing and characterizing phase-controlled broadband optics in the extreme-ultraviolet domain, which should facilitate the manipulation of attosecond pulses for applications.

Compression of attosecond harmonic pulses by extreme-ultraviolet chirped mirrors.

In the race toward attosecond pulses, for which high-order harmonics generated in rare gases are the best candidates, both the harmonic spectral range and the spectral phase have to be controlled. We demonstrate that multilayer extreme-ultraviolet chirped mirrors can be numerically optimized and designed to compensate for the intrinsic harmonic chirp that was recently discovered and that is responsible for temporal broadening of pulses. A simulation shows that an optimized mirror is capable of compressing the duration from approximately 260 to 90 as. This new technique is an interesting solution because of its ability to cover a wider spectral range than other technical devices that have already been proposed to overcome the chirp of high harmonics.

Enhancement of high-order harmonic generation at tuned wavelengths through adaptive control.

An adaptive learning loop enhances the efficiency and tuning of high-order harmonic generation. In comparison with simple chirp tuning, we observe a broader tuning range and a twofold to threefold enhancement in integrated photon flux in the cutoff region. The driving pulse temporal phase varies significantly for different tunings and is more complicated than a simple chirp. We compare our experimental results with a one-dimensional, time-dependent model that incorporates the intrinsic atomic response, the experimental pulse temporal phase, ionization effects, and transverse coherence of the spatial mode of the laser. The model agrees with our experimental results and indicates that a specific quantum path coupled with ionization effects determines the optimized harmonic spectrum.